Unexpected formation of the nickel seco-tribenzoporphyrazine with a tribenzotetraazachlorin-type absorption spectrum.

نویسندگان

  • Victor N Nemykin
  • Anna E Polshyna
  • Elena A Makarova
  • Nagao Kobayashi
  • Evgeny A Lukyanets
چکیده

Minor products in the reaction between substituted 1,3-diiminoisoindolines and 2,5-diamino-3,4-dicyanothiophene were identified as the nickel seco-tribenzoporphyrazines 4 and 5, which have been characterized by UV-vis, MCD, NMR, and mass spectroscopy. Experimentally observed tetraazachlorin-type UV-vis spectra of new seco-tribenzoporphyrazines were explained on the basis of DFT and TDDFT calculations.

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عنوان ژورنال:
  • Chemical communications

دوره 48 30  شماره 

صفحات  -

تاریخ انتشار 2012